ABSTRACT
We present a general approach for studying the dynamics of domain walls in biaxial ferromagnetic stripes with functionally graded Dzyaloshinskii–Moriya interaction (DMI). By engineering the spatial profile of the DMI parameter, we propose the concept of a diode, which implements the filtering of domain walls of a certain topological charge and helicity. We base our study on the phenomenological Landau–Lifshitz–Gilbert equations with additional Zhang–Li spin-transfer terms using a collective variable approach. In the effective equations of motion, the gradients of DMI play the role of a driving force, which competes with the current driving. All analytical predictions are confirmed by numerical simulations.
Topological spin textures have ignited a growing interest in spintronics due to their rich phenomenology,1 as well as novel potential applications. Their nanoscale size and topologically protected stability make them attractive candidates for information carriers in high-density data-storage technologies. For example, domain walls (DWs) and skyrmions in magnetic nanostripes are proposed as key elements of nonvolatile magnetic logic2 and memory3 devices. A diode being the central element of many logical structures is of special interest. Recently, the concepts of ferroelectric domain-wall diode4 and spin-wave diode5 were proposed. Magnetic systems with functionally graded internal material parameters are particularly promising for this use. Recently, spatial engineering of the anisotropy6 and Dzyloshinskii–Moriya interaction (DMI)7 profiles have been suggested as an alternative way of DW and skyrmion guidance and manipulation. The interest in these results is stimulated by the fact that systems with functionally graded material parameters can be fabricated experimentally. For instance, it has been shown that the Bloch DMI can be controlled by the chemical composition8 in chiral ferromagnetic materials. On the other hand, the Néel DMI in multilayer thin films can be tuned by the thickness of the Pt layer,9 the thickness of the ferromagnetic layer,10 electric field,11 and by ion irradiation.12
In this paper, we study the current-induced dynamics of DWs in a chiral ferromagnetic film with functionally graded DMI. We show that the gradient of DMI parameter results in the driving force for DWs similarly to the curvature gradient in wires13 and stripes.14 Considering the coordinate-dependent DMI parameter, we propose a general approach valid for an arbitrary profile of the DMI parameter distribution. We also show how the competition of DMI-induced driving force and current pumping can be potentially used in applications.
We consider a thin and narrow ferromagnetic stripe whose thickness and width are small enough to ensure the one-dimensional character of changes in the magnetization, and the stripe length significantly exceeds the lateral dimensions. Thus, the magnetization is described by a continuous and normalized function , where Ms is the saturation magnetization, x-axis is orientated along the stripe, and t denotes time. The magnetization dynamics is described by the Landau–Lifshitz–Gilbert equation with additional Zhang–Li spin-torque terms,15
where determines the characteristic timescale of the system, with γ0 being the gyromagnetic ratio. Here, is the normalized total energy of the system, where K > 0 is the easy-axis anisotropy constant; see Fig. 1(a). The driving strength is represented by the quantity , which is close to the average electron drift velocity in the presence of a current of density . Here, P is the rate of spin polarization, is the Bohr magneton, and e is the electron charge. Constants α and β denote the Gilbert damping and the nonadiabatic spin-transfer parameter, respectively.
| (1) |

FIG. 1. (a) DW in a biaxial stripe; e.a. and e.p. denote “easy axis” and “easy plane,” respectively. (b) and (c) Possible regimes of DW motion: (b) DW is freely moving, while in (c), DW is pinned. The gray surface in (b) and (c) demonstrates the profile of the DW DMI energy as a function of the DW position q(t) (orange balls correspond to the DW position at different moments of time ), p and are the DW topological charge and helicity, respectively, and d is the dimensionless DMI parameter.
To write the energy functional , we consider a simple model, which takes into account only three contributions to the total magnetic energy
where is the stripe cross sectional area. The first term in (2) is the exchange energy density . The competition between exchange and anisotropy results in the magnetic length , which determines a length scale of the system; here, A is the exchange constant and K is the easy-axis anisotropy constant. The second term in (2) corresponds to the biaxial anisotropy contribution , where , with being the easy-plane anisotropy coefficient. The easy-axis is perpendicular to the stripe plane (xy-plane), while easy-plane coincides with the xz-plane; see Fig. 1. Such kind of anisotropy is effectively induced by the magnetostatic interaction in the thin stripes, with the perpendicular easy-axis magnetocrystalline anisotropy.16 For thin and narrow stripes, the approximation of the shape anisotropy is also used for inhomogeneous magnetization states,17 in particular, DWs.14,18 The last term in (2) corresponds to the Néel DMI , and D(x) describes the spatial profile of the DMI strength. This type of DMI is taken in the form typical for ultrathin films,19,20 bilayers,21 or materials belonging to the Cnv crystallographic group.22
| (2) |
Since , it is convenient to proceed to the angular representation , where and are the magnetic angles. In terms of angular parametrization, the energy density in (2) has the following form:
Here, and below, prime denotes the derivative with respect to the dimensionless coordinate , and is a dimensionless DMI parameter.
| (3) |
Let us first analyze the static magnetization distribution determined by the minimum of the energy (2). Minimization of (2) with associated energy density (3) with respect to results in a solution23 . Here, is a helicity parameter, which determines the orientation of the longitudinal magnetization component mx. This means that vectors m lie within the xz-plane. The corresponding function θ is determined by a driven pendulum equation (see the supplementary material),
Equation (4) is analogous to one, which determines the DW structure in flat curved wires13 and stripes,14 where curvature results in a coordinate-dependent effective DMI.
| (4) |
For the case , Eq. (4) has a well-known DW solution , where q is the DW position, being the topological charge (: kink, p = −1: antikink), and Δ is the DW width. Here, q and Δ are the dimensionless quantities measured in units of . For the case , an additional driving force appears similarly to the case discussed in Refs. 13 and 14. In the following, we consider a case of the spatial distribution of the DMI strength, with , which allows the boundary conditions . We restrict ourselves to the case and consider as a small perturbation, which does not significantly modify the profile of the DW and its width Δ. Therefore, to analyze the DW properties, we use the collective variable approach based on the q– model,24,25
Here, are the time-dependent conjugat collective variables, which determine the DW position and phase, respectively. The DW width Δ is assumed to be a slaved variable,16 i.e., .
| (5) |
Substituting the Ansatz (5) into (3) and performing integration over the ξ coordinate, we obtain the energy of a DW in the stripe in the form
where the condition was imposed when integrating (2). The structure of the energy (6) has similar form as DW energy in stripes with constant DMI strength26,27 and in a curved biaxial stripe.14 The first two terms on the right-hand side in (6) determine the competition of the isotropic exchange and anisotropy contributions, while the third term originates from the DMI and demonstrates the coupling between the DMI strength d, DW topological charge p, and helicity ; i.e., DMI energy is minimized when . The coupling between DMI and DW topology determined by p and was previously indicated in Ref. 28. In the following, a DW, which corresponds to the global minimum of the energy (6) in the parametric space , is called stable. Under the condition , energy (6) also has a local minimum, which corresponds to a DW with the opposite helicity . In the following, this DW is called metastable.
| (6) |
In terms of collective variables, the equations of motion (1) take the form (see the supplementary material)
where overdots indicate the derivative with respect to the dimensionless time , and is a dimensionless current. The DW width is . The behavior of the DW width is discussed in detail in the supplementary material.
| (7) |
For the case , Eq. (7) coincide with the equations of motion for DW in a curved biaxial stripe presented in Ref. 14, with the curvature gradient replaced by the gradient of the DMI strength. The DMI-induced driving force can suppress the action of the pumping by the spin-polarized current or can reinforce it; see Fig. 2. In other words, the metastable (stable) DW has to overcome the energy barrier when it enters the region with larger (smaller) . If the applied current is small enough, then such a DW is pinned in position . For small currents, the phase of the pinned DW does not significantly deviate from its equilibrium value: . The average DW velocity as a function of current for the DMI profile with amplitude d0 and width w is presented in Fig. 2(a); also see the supplementary material movies for the corresponding DW dynamics. Zero averaged velocity29 corresponds to the case of pinning.

FIG. 2. (a) Averaged DW velocity as a function of the applied current. Solid lines correspond to solutions of the collective variable equations (7). Dashed lines correspond to DW velocity (9). (b) and (c) Eigenfrequency of DW oscillations in the vicinity of the pinning position. Solid and dashed lines are plotted with prediction (S11) (see the supplementary material) and its approximation for zero damping and small currents (8), respectively; filled gray area in (b) and (c) corresponds to the overdamped regime when DW is pinned without oscillations with Ω = 0; filled yellow area corresponds to the currents with . (d) The eigenfrequency of DW oscillations in the vicinity of the pinning position in terms of density plot. Solid line corresponds to the depinning current . Symbols in (a) and (b) correspond to the numerical simulations with ; see the vertical dashed line in (d). All other parameters of simulations: , w = 10, and stripe width . In (b)–(d), we have .
The behavior of DW velocity presented in Fig. 2(a) demonstrates that functionally graded DMI allows filtering of DWs of a certain type; i.e., we have built a DW diode in a planar nanostripe.30 Depinning of DWs takes place when current exceeds some critical value ; see Fig. 2(d).
Next, we study the linear dynamics of the DW in the vicinity of the DW pinning position. With this purpose, we introduce small deviations as and . The equations of motion (7) linearized with respect to the deviations read as , where and matrix depends on current (see the supplementary material). For the case of low damping and low current, we have decaying oscillations with frequency
The frequency Ω as a function of the applied current is plotted in Figs. 2(b) and 2(d). Depinning of the DW takes place for cases (i) [see Fig. 2(b)] or (ii) . In the latter case, the metastable DW experiences the phase flip and transforms into the stable DW. The limiting case of does not produce any pinning due to the zero gradient of the DMI strength.
| (8) |
Now, we consider the case with zero gradient of the DMI strength, i.e. . For this case, Eqs. (7) have a solution for the traveling-wave regime, with and (the case is discussed in Ref. 15). The corresponding DW velocity and phase (in the small current approximation) are
It is necessary to mention that the DW velocity (9) is independent of the DMI parameter and coincides with the DW velocity reported in Ref. 15; see Fig. 2(a). The traveling-wave solution (9) exists for the currents , where
Here, “+” sign corresponds to the stable DW, while “−” sign corresponds to the metastable DW, and is the Walker current for the DMI-free biaxial ferromagnetic system.15 Estimation (10) is obtained under the assumption . From (10), it follows that the DMI results in the shift of the Walker current in the biaxial stripe similarly to the case of field-driven DW.31 The value of the Walker current for metastable DW is smaller as compared to that of the stable one and it defines the current of the DW phase flip; i.e., for , we have traveling-wave motion with a single flip of the phase with [see Figs. 3(b) and 3(c)]. One should note that for the case , both DWs move in a traveling-wave regime without any flip of the phase , i.e., . The average DW velocity as a function of current is presented in Fig. 3.
| (9) |
| (10) |

FIG. 3. (a) Averaged velocity of a stable DW as a function of the applied current. Lines correspond to solutions of the collective variable equations (7) with , and symbols show the results of numerical simulations. Dashed lines correspond to the Walker current (10). (b) and (c) show evolution of for DW for different values of current in terms of density plot for stable and metastable DWs, respectively [data obtained from solutions of the collective variable equations (7) with and ]. In all simulations, we use , and stripes of width .
Let us estimate the effective mass of the DW.32 To this end, we consider a no driving case (u = 0) with vanishing damping. In this case, a small deviation of the DW phase from its equilibrium value results in the traveling-wave DW motion with the velocity . Using the latter relation and energy expression (6), one can estimate the energy of the moving DW as , where is the energy of a stationary DW, and the quantity can be interpreted as the effective mass of the DW. For the DMI-free case (), the effective mass μ coincides with the Döring mass.32 The DMI results in the modification of the DW mass; i.e., for stable (metastable) DW, the mass μ decreases (increases) with the DMI strength.
We have demonstrated that the presence of the biaxial anisotropy () and DMI () allows the existence of DWs with different combinations of topological charge and helicity (). One of these DWs becomes energetically preferable (stable DW); i.e., it minimizes the DMI energy . By engineering the profile of the DMI strength, the stable DW will move to the area with a larger DMI strength and will be pinned for the opposite direction, while behavior for the metastable DW is vice versa. This effect can be used for the fabrication of a DW diode, traps, and ratchets in a planar stripe. These can be potentially used for the development of logic devices. We show that the gradient of functionally graded DMI in magnetic systems results in the driving force for DWs. The competition between the DMI driving force and pumping by the current determines the behavior of DW dynamics. The intrinsic DMI results in the shift of the Walker current (10), which allows us to increase the maximal velocity of traveling-wave motion for the DW; DMI modifies the DW Döring mass μ. This shows that functionally graded materials open new possibilities in the manipulation of DWs. We expect that similar pinning effects can appear for magnetic skyrmions as well.
See the supplementary material, which contains details of analytical calculations, numerical simulations, and movies.
We thank U. Nitzsche for technical support. K.V.Y. acknowledges financial support from UKRATOP-project (funded by BMBF under Reference No. 01DK18002). J.B. acknowledges support from the German Research Foundation (Deutsche Forschungsgemeinschaft, DFG) via SFB1143 project A5 and through the Würzburg-Dresden Cluster of Excellence on Complexity and Topology in Quantum Matter-ct.qmat (EXC 2147, Project ID 39085490). In part, this work was supported by the Program of Fundamental Research of the Department of Physics and Astronomy of the National Academy of Sciences of Ukraine (Project No. 0116U003192), by the Alexander von Humboldt Foundation (Research Group Linkage Programme), by the Taras Shevchenko National University of Kyiv (Project No. 19BF052-01), and by the U.S. Department of Energy.
DATA AVAILABILITY
The data that support the findings of this study are available within the article and its supplementary material.
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