ABSTRACT
We fabricated MnBi2Se4/(n − 1) quintuple layer (QL) Bi2Se3 magnetic topological heterostructures (n = 1–6) and measured the Dirac cone dispersion with angle-resolved photoemission spectroscopy. We observed a clear gap opening for films with n = 2–6 and the gap size decreased as the film thickness increased. From magnetization measurements using SQUID, all the heterostructures showed hysteresis loops at 4 K and at room temperature, confirming that MnBi2Se4 is a room temperature van der Waals ferromagnet. We were able to distinguish the contribution of the hybridization and magnetic effects on the observed Dirac-cone gap directly using a four-band model and its implications on the behavior of the expected quantum anomalous Hall effect is discussed.
The authors thank S. Ichinokura and R. Akiyama for the discussions. The authors also thank Y. Tomohiro for the assistance in the magnetization measurement using SQUID. This work has been supported by the Grants-In-Aid from Japan Society for the Promotion of Science (No. 18H03877), the Toray Science Foundation, the Murata Science Foundation, the Asahi Glass Foundation, and the research support from the Tokyo Institute of Technology.
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